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Charles McCombie ARIUS: Association for Regional an International Underground Storage 5405 Baden/Switzerland Introduction In this symposium on technology and policy issues associated with nuclear wastes, I have been asked to address specifically three key issues: reprocessing, storage and disposal. Before doing so, I will give a brief, but quantitative, overview of the nuclear fuel cycle in order to illustrate which wastes arise from the activities involved therein. Following this I will try to overview the status of technologies for storage, reprocessing and disposal and to address key policy issues associated with each of these technologies. The technical maturity and development potential differ strongly between the three fields, as do the political and societal issues currently being debated in each case. The nuclear fuel cycle and its wastes The conventional fuel cycle begins with mining or in-situ leaching of uranium ores (containing typically 0.15 to 0.2% uranium, but sometimes much higher - up to 20%) which are then concentrated and processed to produce uranium oxide (U3O8 "yellow cake").This oxide passes through a conversion plant, the product of which is uranium hexafluoride (UF6), which is fed to an enrichment plant. Here the content of the fissile isotope U235 is increased from its natural level of 0.7% to around 3-5%, with 85% of the feedstock being rejected as depleted uranium or tails. The enriched uranium goes to a fuel fabrication plant where it is converted to UO2 and incorporated into fuel assemblies. For a 1000 MWe, light water reactor (LWR), with around 80t of fuel is in the core at any time with a fraction being replaced each year. At a high burn-up of 50GWd/tU, this fuel will produce a total of around 3.3 GW.a of electricity. During its years in the reactor each tonne of fuel will, from the U235 and U238 that are fissioned, produce around 60kg of fission products, 10kg of plutonium isotopes, and 8 kg of U236 and various other transuranics. If the spent fuel is reprocessed, then the fission products are solidified to yield around 50l of vitrified high level waste (HLW). A 100MWe nuclear power station therefore produces only 10-20 canisters of vitrified waste per year. The material flows and, importantly, the waste production are summarised in Figure 1. Figure 1: Typical material flows in fuel cycles All of the operations listed produce radioactive wastes in solid, liquid or gaseous forms. The greatest environmental challenges may actually be associated with wastes at the front end of this chain - namely managing safely the millions of tonnes of mining and milling tailings that remain on or near the land surface of uranium producing countries. However, most time, effort, resources and public attention are devoted to management of the low volume but highly hazardous wastes from the back-end of the fuel cycle. These are spent nuclear fuel (SNF), if this is regarded as waste, or the vitrified HLW ( and the accompanying transuranic wastes that are produced if a reprocessing route) is chosen. This paper also concentrates on the technical and policy issues associated with storing and disposing of these two waste streams. As far as disposal is concerned, this implies that the discussion will focus on deep geologic repositories, since these are recognised as being the only feasible method today of achieving safe permanent disposal. Technical and policy issues The title of this symposium highlights the fact that in the nuclear field there is an especially strong connection between technical and policy issues. Nuclear technology discussions in our society today tend to be highly polarised with committed exponents of extreme views on both the benefits and the drawbacks. There have been various explanations put forward for this: the military origins of advanced nuclear technology, the long-continued secretive approach of the civilian nuclear industry, the largely unprecedented scale of potential positive and negative consequences, an innate or inherent dread of unseen hazards, a reaction against all new and large scale technologies, etc. It is not the place here for detailed examination of such ideas. It is important, however, to be aware that the unusually controversial debate on nuclear matters can affect directly the judgement of debaters on both technical policy and issues associated with nuclear applications. For the three areas proposed for comment, storage, reprocessing and disposal, Table 1 gives a concise summary of my assessment of the primary technical and policy points to be made. Those cognoscenti who are familiar with current debates on these activities can read from the table most of the messages I wish to present. For those less intimately involved in the technologies, each point is discussed individually below. Because of my personal experience and interests, but also because it is currently the most controversial issue, more discussion is devoted to waste disposal than to the other two topics. Storage of nuclear wastes I begin by looking at the technological and policy issues associated with storage because this is the simplest of the three activities to be addressed. Storage of wastes is a long-established technology; it is widely practiced today and will continue to be necessary for many decades into the future, since no subsequent technology that removes the need for continuing storage will be implemented for a long time. The HLW and SNF upon which we are concentrating are extremely radioactive for many years. The SNF contains fissile materials that could potentially be misused in nuclear weapons. The radiological hazards associated with both waste types are very high, so that reliable measures are needed to ensure that there is no inadvertent entry of radionuclides into the environment and that deliberate releases by malevolent groups are excluded. In short, safety and security of stored HLW and SNF must be guaranteed. The technologies for safe storage are well proven. Early storage facilities for SNF were primarily in water pools in well protected nuclear facilities (wet storage). Increasingly, spent fuel and HLW is being stored in strong sealed and shielded containers (dry storage) or in vaults. Both wet and dry approaches can provide safety and security. The dry storage approach is better suited for very long storage periods, although some wastes (e.g. SNF from Magnox reactors) must be kept under water for safety reasons. No technical developments are necessary for ensuring the safety of storage (although work is still going on examining fuel creep, hydrogen migration etc.). The recent rise in terrorist acts has led to some re-examination of security aspects, such as susceptibility to missile attack. In most countries, spent fuel is stored in pools at the reactor site. In some, e.g. Sweden and Finland, centralised pool storage has been implemented. Dry storage casks have been licensed at reactor sites in the USA and Canada, centralised cask stores are in operation in Germany and Switzerland, and dry storage in vaults is practised in the UK. Storage is technically unproblematic; but there are some important policy issues to be addressed. These concern the duration and the location of storage activities. When reactors or reprocessing plants were built it was believed that the SNF or HLW would be removed (after limited storage to allow cooling) and shipped to a disposal facility. The huge delays in implementing such facilities have meant that storage periods are drastically extended; in some countries geologic repositories are so distant that no date is predictable; in a few countries there is insufficient acceptance of the feasibility off geologic disposal so that storage becomes "indefinite". These policy positions have some feedback to technical issues such as long-term maintenance, replacement of obsolete facilities, etc. However, the key issues are societal. Communities currently hosting SNF or HLW stores or being proposed as hosts do not wish to become de-facto final repositories. This controversy is growing with time, since the delays in disposal are leading to increasing requirements for storage. The additional storage can be at reactor sites., providing licenses can be amended, or at new centralised storage facilities, providing these can be sited. Extending storage at operating sites (by introducing compact storage in existing pools or by expanding facilities) is proving feasible in various countries; in others, for example the USA and Taiwan, reactor operators are having increasing problems. What will happen if the need for storage outlasts the operational lifetime of the facility is unclear. In Germany the anti-nuclear government has introduced a deliberate policy of implementing at-reactor storage, although existing centralized facilities are not been utilized. This is based on the unjustified assertion that transport risks rule out transfer to the existing stores. In practice, German transports have been made enormously complex and expensive because of the measures needed to control the extensive public opposition (which is targeted on specific transfers to the Gorleben site)). In the USA, because some reactor operators cannot implement sufficient on-site storage of SNF, contentious litigation has been initiated with the USDOE, which failed to meet its 1998 target date for acceptance of such fuel. This has also led to proposals for storage facilities run as private enterprises. The situation in the USA concerning storage and disposal illustrates well how policy issues can directly affect technical programmes. To run disposal operations as efficiently as possible it would be advantageous to have a large storage capacity close to the repository so that waste emplacement could be decoupled from acceptance and could be planned to minimise thermal loading problems. The newly published study of repository staging by the National Research Council also makes this point for the Yucca Mountain Programme. Because of the political sensitivities associated with implementing large stores before repositories are available, this is currently not a feasible policy option in most countries. One solution would be that the host community agrees contractually with the operator of the storage facility that the wastes must be removed by a certain date. This is the case with the Swiss ZWILAG storage facility - however, long-term contracts of this nature require a level of mutual trust that is not always in evidence between communities and implementers. Reprocessing of spent fuel Civil reprocessing technology was developed in order to obtain unused uranium and plutonium for use in fast reactors. The technical challenges associated with the process have been solved and reprocessing plants have run on a large scale in France, the UK, Russia, the USA, and in other countries (e.g. Belgium and Italy) as research operations. France, the UK and Russia offer commercial reprocessing services that a number of countries are using or have used (e.g. Japan, Germany, Switzerland, Italy, Spain and Sweden). Japan is currently building its own commercial plant. The technology of reprocessing spent fuel with separation of plutonium and recovery of unused uranium is established. Technical improvements could increase separation efficiencies or could reduce emissions of radioactive substances during operation. There are bigger technical challenges, however. One is to develop an advanced reprocessing and fuel fabrication cycle that avoids having segregated plutonium at any stage. This could greatly reduce the proliferation risks associated with reprocessing. Another technical challenge might be to develop a "second generation" waste form to replace the borosilicate glasses in which the fission products are included at present. Much work has been done on development of ceramics and synthetic minerals. Whether the improved performance that these can show is needed in order to further increase the high levels of safety already predicted for repositories is the main question. In fact, the main technical challenge associated with reprocessing may actually be associated with the mundane goal of reducing costs. Currently the costs of reprocessing are so high that they cannot be compensated by the value of the recovered materials nor by the savings on spent fuel storage and disposal costs. Using estimated figures for reprocessing costs of around USD 1000/kg and mixed oxide fuel fabrication costs of USD 2000/kg give, for the production of 1 kg of mixed oxide (MOX) fuel, a cost of USD 7000, since recovered material from 5 kg of uranium fuel is needed. Savings are achieved by not having to dispose of these 5 kg of uranium but these are not sufficient to offset the price differential to uranium fuel, which costs around USD 1400/kg. Commercial break-even would happen only if the price of the 8 kg of uranium feed increased far beyond the current typical uranium prices of 20-40 USD/kg. Another driver that could make MOX fuel commercially more attractive would be if subsidies could be given for MOX fuel use because of its potential value in eliminating excess weapons plutonium. This major technical challenge of reducing reprocessing costs is intimately connected with the policy reasons that originally led to development of the technology. A once through fuel cycle burning U235 utilises about 3.5% of the fission energy in the uranium; reprocessing and use of plutonium in fast reactors could allow 60-90% to be used. The policy decisions that led to development of commercial reprocessing were, therefore, based upon the desire to conserve uranium resources by providing a plutonium supply for fast reactors. This argument has been severely weakened over time by the fact that the slow growth of nuclear power has meant that uranium has remained cheap. Moreover, postponed deployment of breeders has reduced demand for, and therefore value of, plutonium. In fact, the excess plutonium already produced from reprocessing has become a liability (it is expensive to store and degrades in storage) and represents a potential proliferation risk. Today the nuclear industry is using some plutonium in MOX fuels, although the costs are high (as mentioned above) and the uranium savings only around 20%. Serious consideration is therefore being given to reactors designed for deliberately burning excess plutonium and even to directly disposing of plutonium as a waste. In summary the key policy issues associated with reprocessing are the weakened resource conservation arguments, the increasing concerns about nuclear proliferation and the non-viable economics when fresh uranium can be extracted at low prices. Indeed, it has been argued that the prices of extracted uranium would have to rise to some hundreds of USD/kg to make reprocessing commercially competitive - and at such prices it may even be feasible to extract effectively unlimited quantities of uranium from sea water. Countries that currently follow a reprocessing strategy do so for one or more of the following reasons: